To clean the valve faces and cylinder area of the cylinder head, I use a wire wheel in the drill.
Go easy here because you don't want to dig in, just clean it and keep the wire wheel off the gasket surface.
Well you could run the wheel on the gasket surface but feel is important here which is why I usually don't recommend it. Don't let it gouge or dig into the aluminum. The aluminum is pretty tough but still........go easy while you get a feel for it.
There are wire wheels with softer wire so they flex some, get one of those.
Then on to the cylinders but don't use a wire wheel here.
Depending the condition will determine which way to clean them.
Is there any pitting in the cylinder walls?